King Shark? Been on the Suicide squad, as well as being a shared villain with Superboy
The Shark. Shared villain of both Aquaman and Green Lantern
The Eel recently appeared in Mera’s mini
Scavenger is a big named Aquaman villain
Atlan the Dead King was a really good one
Siren? Could be considered an Aquaman villain
I could list a bunch Charybdis, Marine Marauder, Creature King, Deadwater, The Giant Born, Fire Trolls, Thule, Gamamnae, The Thirst being the ones off the top of my head