For me, Batman Begins: probably the only Batman non-animated film I've seen in which I find Batman himself to be a compelling character.
In some ways, I think Batman '89 and The Dark Knight share the same problem: the villain overpowers the movie, and is more compelling, interesting, and charismatic than the main protagonist. They're good Joker films - whether you prefer Joker as a psychotic gangster or as an agent of chaos, respectively - but not great Batman films. (The Dark Knight, in addition, is hampered by the preposterous Bat Voice.) That's true of some of the other Bat films IMO - Batman Returns and Batman Forever, both entertaining films with good villains (Jones' misfiring Two Face aside) - although oddly enough not true of Batman and Robin, although that's purely because Ivy, Bane and Freeze are so catastrophically bad
Part of the reason, I tend to think, is that visually Batman as a character works wonderfully in the comic and in animation, but nowhere near as well in the non-animated movies.
Batman '66 I find didn't capture the magic of the series, and I haven't seen The Dark Knight Rises.