Thor
Captain America
Ironman
I feel like I'm the only guy that likes the Thor movies. They aren't the best Marvel films but they have enjoyable moments.
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Easily the best.
Iron Man started the MCU off with a huge bang, but since then the concepts that seemed like they were tailor made for the big screen have really been pretty lackluster. Iron Man 2 & 3 were disappointing misses. Thor and The Incredible Hulk were decent enough but really had messy 3rd acts, and a lackluster, forced villain in the case of TIH. Thor 2 and Ant-Man were uneven results of production/director issues.
I mean, Cap has been the best by default to this point, it's fortunate for the genre that his movies have been so good. TFA was better than it had any right to be, given the need to connect the comic book trappings to WWII, and I thought for sure they would completely botch Red Skull and they didn't. Winter Soldier was incredible in about every way. Civil War managed to even top that though. And yes, I thought the Cap-Bucky thread managed to play well throughout and make it feel as if it was a Cap movie at its core that happened to guest star Iron Man and feature the Avengers in extended cameo, and didn't come off as "Avengers 2.5" at all.
The Incredible Hulk is my favorite.
But I'd give The Winter Soldier second place.
TRUTH, JUSTICE, HOPE
That is, the heritage of the Kryptonian Warrior: Kal-El, son of Jor-El
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Iron Man for me.
But I would also argue that other than the first one, Captain America hasn't had any solo movies even if it was his name in the title. I can't see Winter Soldier and Civil War as solo movies.
I think Hemsworth has been badly underrated in his contributions (particular in the first Avengers movie). Hiddleston did a nice job in the first Thor movie, but I haven't been particularly impressed with him since then. Although, in the case of Avengers, I think that's largely the result of him being given a badly underwritten part (although he still managed to chew the scenery with gusto, nonetheless).
TRUTH, JUSTICE, HOPE
That is, the heritage of the Kryptonian Warrior: Kal-El, son of Jor-El
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This.
I've never been much of a CA fan in the comics - but I absolutely loved him in the movies. Chris Evans is perfectly cast, Seb Stan a wonderful Bucky and an even better WS, and CA2WS is the only film I actually liked Black Widow in.
These films had heart and soul and a leading character you could really care about. Sadly, the Thor movies completely wasted Norse myth except for Loki, and IronMan never topped the first film although they were enjoyable.
The Winter Solider was/is. First Avenger wasnt very good at all, and Civil War was an Avengers film.